Strüber, Christian: Ultrafast coherent control and multidimensional spectroscopy on the nanoscale. 2014
Inhalt
- Publications
- Preface
- Introduction
- Basic Theoretical and Experimental Concepts
- Description and Representation of Polarization-Shaped Laser Pulses
- Temporal and Spectral Description of Femtosecond Laser Pulses
- Spatial Propagation of Light in Dispersive Media
- Elliptical Pulse Parameter
- Concepts of Laser Pulse Shaping
- Polarization Pulse Shaper Setup
- Methods for Amplitude, Phase and Polarization Pulse Shaping
- Adaptive Techniques for Pulse Shaping
- Optical Near-Fields and Optical Nanoantennas
- Localization of Light below the Diffraction Limit
- Propagating Surface Plasmon Polaritons
- Localized Surface Plasmon Resonances
- Nanoantennas and Coupling of Plasmonic Modes
- Spatial and Temporal Control Mechanisms
- Time-Resolved Photoemission Electron Microscopy
- Optimal Open-Loop Near-Field Control of Plasmonic Nanostructures
- Introduction
- Experimental Setup and Sample Characterization
- Open-Loop Control of Nanoplasmonic Excitations
- Conclusion
- Spatially and Temporally Resolved Control of Nanooptical Excitations
- Introduction
- Experimental Setup and Sample Characterization
- Ultrafast Nanoscale Excitation Switching
- Conclusion
- Principles of Coherent 2D Nanoscopy
- Bringing Nonlinear Spectroscopy to the Nanoscale
- Principles of Coherent 2D Nanoscopy
- Liouville Space Description of 2D Nanoscopy
- 2D Nanoscopy in Strongly Dephasing Systems
- 2D Nanoscopy for Single Harmonic Oscillators in Strongly Dephasing Systems
- Phase Cycling
- Simulation of Coherent 2D Nanoscopy
- Hybridization of Dark and Bright Plasmonic Modes
- Experimental Setup and Sample Characterization
- Optical Near-Field Control of Hot Spot Photoemission on Silver
- Near-field Superenhancement
- Sub-Diffraction Control of Photoemission Hot spots
- Reproducibility of Adaptive Optimizations
- Multidimensional Pulse Parameter Scans
- Conclusion
- Coherent 2D Nanoscopy on a Corrugated Silver Surface
- Hybridization of Plasmonic Modes on a Corrugated Ag Surface
- Localization of Photonic Modes in Thin-Film Solar Cells
- Hydrogenated Amorphous Silicon Thin-Film Solar Cells
- Sample Characterization
- Sample Designs and Structural Properties
- Linear Absorption Spectroscopy
- Ultrafast Backscattering Spectroscopy Experiments
- 2D Nanoscopy on Nanotextured Thin-Film a-Si:H
- Nonlinear Hot Spot Electron Emission from Nanotextured a-Si:H
- Thermionic Emission from Photonic Mode Heated Hot Spots
- 2D Nanoscopy on Nanotextured Thin-Film a-Si:H
- Conclusion
- Summary and Outlook
- Laser Pulse Characterization
- Experimental Pulse Characterization
- Jones-Matrix Formalism
- Jones-Matrix as Pulse Characterization Tool
- Drift Correction of PEEM Data
- Excitation Pathways for Single Color Pump-Probe Experiments
- Principles of Optical Coherent 2D Spectroscopy
- Representation of Mixed Quantum Mechanic States with the Density Matrix
- Response Function Formalism in Liouville Space
- Liouville Pathways for Third Order Polarization
- Optical 2D Spectroscopy in Experiments
- 2D Nanoscopy: Mathematical Details
- Local Photoemision Rate for n=4 in Explicit Notation
- Partial Photoemission Rate for Lorentz Oscillator Response Function
- Lorentz Oscillator
- List of Figures
- Bibliography
- Acknowledgements